non-linear optics非线性光学

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1、NONLINEAROPTICSLECTURENOTES2001Prof.W.UBACHSLASERCENTREVRIJEUNIVERSITEITAMSTERDAMDEPARTMENTOFPHYSICSANDASTRONOMYContentsCh1:Non-linearoptics:Introduction1.1THEFIRSTOBSERVATIONOFANONLINEAROPTICALPROCESS11.2THENONLINEARSUSCEPTIBILITY11.3GRAPHICALREPESE

2、NTATIONOFNONLINEAROPTICS21.4LORENTZMODELOFTHESUSCEPTIBILITY31.5MAXWELL’SEQUATIONSFORNONLINEAROPTICS61.6THECOUPLEDWAVEEQUATIONS71.7NONLINEAROPTICSWITHFOCUSEDGAUSSIANBEAMS9Ch2:Secondharmonicgeneration2.1SECONDHARMONICGENERATIONANDPHASEMATCHING132.2WAVE

3、PROPAGATIONINANISOTROPICMEDIA;INTERMEZZO162.2aREFRACTIONATABOUNDARYOFANANISOTROPICMEDIUM192.2bTHEINDEXELLIPSOID192.3THENONLINEARCOEFFICIENT222.4PHASEMATCHINGINBIREFRINGENTMEDIA242.5OPENINGANGLE262.6PHASEMATCHINGBYANGLETUNING282.7PHASEMATCHINGBYTEMPER

4、ATURETUNING292.8QUASIPHASEMATCHINGBYPERIODICPOLING302.9PUMPDEPLETIONINSECONDHARMONICGENERATION33Ch3:Theopticalparametricoscillator3.1PARAMETRICAMPLIFICATION363.2PARAMETRICOSCILLATION373.3TUNINGOFANOPO383.4BANDWIDTHOFTHEOPO413.5PUBLICDOMAINSOFTWARE42C

5、h4:Quantumtheoryofthenonlinearsusceptibility4.1SCHRODINGEREQUATION;PERTURBATIONTHEORY434.2CALCULATIONOFPROBABILITYAMPLITUDES454.3FIRSTORDERSUSCEPTIBILITY464.4SECONDORDERSUSCEPTIBILITY474.5THIRDORDERSUSCEPTIBILITY492Ch5:CoherentRamanScatteringinGases5

6、.1THIRDORDERNON-LINEARSUSCEPTIBILITY515.1.1NON-LINEARGAINPROCESSES525.1.2FOUR-WAVEMIXINGPROCESSES525.2SPONTANEOUSRAMANSCATTERING525.3STIMULATEDRAMANSCATTERING535.4FIRSTSTOKESGENERATION555.5RAMANSHIFTIINGINHYDROGEN575.6COHERENTANTI-STOKESRAMANSPECTROS

7、COPY(CARS)58Ch6:TheproductionofvacuumultravioletradiationbyFWM6.1THIRDHARMONICGENERATION636.2PHASE-MATCHINGUNDERFOCUSINGCONDITIONS646.3NUMERICALAPPROACHTOTHEPHASE-MATCHINGINTEGRALS686.4PHYSICALINTERPRETATIONOFPHASE-MATCHINGINTEGRALS706.5OPTIMIZINGDEN

8、SITYINTHENON-LINEARMEDIUM716.6DISPERSIONCHARACTERISTICSOFTHENOBLEGASES736.7THIRDHARMONICGENERATIONINXENON746.8RESONANCE-ENHANCEDVUVUPRODUCTION756.9POLARIZATIONPROPERTIES776.10PULSEDJETS783Chapter1Non-linearoptics:Introduction1.1THEFIRSTOBSERVATIONOFA