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Synthetic routes toward MOF nanomorphologies

Synthetic routes toward MOF nanomorphologies

ID：40372147

大小：1.14 MB

页数：15页

时间：2019-08-01

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1、ViewArticleOnline/JournalHomepage/TableofContentsforthisissueJournalofDynamicArticleLinksC

2、ch*Received5thNovember2011,Accepted17thJanuary2012DOI:10.1039/c2jm15675jAsmetalorganicframeworks(MOFs)arecomingofage,theirstructuraldiversity,exceptionalporosityandinherentfunctionalityneedtobetransferredintousefulapplications.FashioningMOFsintovariousshapesandatthesametimecontrollingthe

3、irsizeconstituteanessentialsteptowardMOF-baseddevices.Moreover,downsizingMOFstothenanoscaletriggersawholenewsetofpropertiesdistinguishingnanoMOFsfromtheirbulkcounterparts.Therefore,dimensionality-controlledminiaturizationofMOFsenablesthecustomiseduseofnanoMOFsforspecificapplicationswheres

4、uitablesizeandshapearekeyprerequisites.InthisfeaturearticlewesurveytheburgeoningfieldofnanoscaleMOFsynthesis,rangingfromclassicalprotocolssuchasmicroemulsionsynthesisallthewaytomicrofluidic-basedtechniquesandtemplate-directedepitaxialgrowthschemes.Alongtheselines,wewillfathomthefeasibility

5、ofrationallydesigningspecificMOFnanomorphologieszero-,one-andtwo-dimensionalnanostructuresandwewillexploremorecomplexsecond-generationnanostructurestypicallyevolvingfromahighlevelofinterfacialcontrol.Asarecurringtheme,wewillreviewrecentadvancesmadetowardtheunderstandingofnucleationandgrow

6、thprocessesatthenanoscale,assuchinsightsareexpectedtofurtherpushthebordersofnanoMOFscience.1.Introductioncomposedofmetalionsorclustersjoinedbyrigid,polytopicorganiclinkers.1,2ThetriumphantsuccessandrapidgrowthofCoordinationchemistryhaslivedthrougharenaissancewiththethisclassofhybridmater

7、ials,dubbedmetalorganicframeworksdiscoveryofhighlyporous,crystallineframeworkmaterials(MOFs)orporouscoordinationpolymers(PCPs),arelargelybasedontheirelegantyetsimplesynthesisandtheirversatilityoriginatingfromtheuseoftailorablelinkersandtheresultingaMaxPlanckInstituteforSo

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