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1、膨胀石墨基炭/炭复合材料的改性及其对甲醛气体的吸附性能研究顾诚1,陈志刚1,2,3,刘成宝2,3,马娟宁1(1.江苏大学材料科学与工程学院,江苏镇江212013;2.苏州科技学院 江苏省环境功能材料重点实验室,江苏苏州215009;3.苏州科技学院 化学与生物工程学院,江苏苏州215009)摘要:首次选用双氧水、硝酸、氨基酸(氨基和羧基的脂肪族有机酸)、氯化铵、CTAB(cetyltrimethylammoniumbromide,十六烷基三甲基溴化铵)等溶液浸渍改性膨胀石墨基炭/炭复合材料(EGCs),考察改性剂的浓度、吸附温度、吸附时间对甲醛气体吸附效果的影响,结果表明,经CTAB溶液
2、改性后,EGCs对甲醛气体的吸附性能得到提高,而经双氧水、硝酸、氨基酸、氯化铵等溶液改性的EGCs对甲醛气体的吸附能力反而下降。当CTAB浓度为0.01mol/L,改性温度为70℃,改性时间为60min时,材料对甲醛的静态吸附效果最好,最高吸附量可达1042mg/g。关键词:甲醛;膨胀石墨基炭/炭复合材料;改性;吸附中图分类号:TQ165文献标志码:AMODIFICATIONOFEXPANDEDGRAPHITE-BASEDCARBON/CARBONCOMPOSITESBYVACUUMIMPREGNATIONANDITSADSORPTIONPROPERTIESONFORMALDEHYDEG
3、uCheng1,ChenZhigang1,2,3,LiuChengbao2,3,ChenFeng1(1.SchoolofMaterialsScienceandEngineering,JiangsuUniversity,Zhenjiang212013,China;2.TheKeyEnvironmentalandFunctionalMaterialsLaboratoryofJiangsuProvince,SuzhouUniversityofScience&Technology,Suzhou215011,China;3.SchoolofChemistryandBiologicalEnginee
4、ring,SuzhouUniversityofScience&Technology,Suzhou215011,China)Abstract:Accordingtopropertiesofformaldehyde,expandedgraphite-basedcarbon/carboncomposites(EGCs)wasmodifiedbyimpregnatingwithsolutionsofhydrogenperoxide,nitricacid,aminoacid,ammoniumchloride,cetyltrimethylammoniumbromide(CTAB)andetc.For
5、maldehydeadsorptionpropertiesofEGCsmodifiedwithdifferentsolutionswerestudied.Andeffectsofmodifiedandadsorptiveprocessesonadsorptionpropertiesforformaldehydegaswereinvestigated.TheresultsshowthatformaldehydegasadsorptionpropertyofEGCsmodifiedwithCTABisbetterthanthatofEGCsnotbeingmodified,whileform
6、aldehydegasadsorptionpropertiesofEGCsmodifiedwithhydrogenperoxide,nitricacid,aminoacid,ammoniumchloride,ureahavedropped.WhenCTABconcentrationis0.01mol/L,modificationtemperatureis70℃,themodificationtimefor60min,thesemodificationconditionsweresuperiortoothersforformaldehydegasadsorption.Meanwhile,t
7、heoptimizedadsorptiontemperaturetoformaldehydegasisinroomtemperature(25℃).Inthisexperiment,theadsorptioncapacityofmodifiedEGCsonformaldehydegaswasashighas1042mg/ginthebestprocesscondition.Keywords:formaldehyde;Expanded