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1、Letterpubs.acs.org/journal/estlcu137ASurveyofCsinSedimentsoftheEasternMediterraneanMarineEnvironmentfromthePre-ChernobylAgetothePresentNikolaosEvangeliou,*HelenyFlorou,andPanayotisKritidisNationalCentreforScientificResearch“Demokritos”,InstituteofNucleara
2、ndRadiologicalSciencesandTechnology,EnergyandSafety,EnvironmentalRadioactivityLaboratory,,15310Athens,Greece*SSupportingInformationABSTRACT:Asurveyof137CsinsedimentsfromtheeasternMediterraneanSea(AegeanandIonianSeas)duringtheperiodfrom1984to2007ispresent
3、ed.DatahavebeencollectedandanalyzedintheframeworkofthemonitoringsystemofGreeceperformedbytheEnvironmentalRadioactivityLaboratory(NCSR“Demokritos”)overthepast30years.SedimentactivitiesreflecttheimpactfromtheChernobylaccidentoneyearlater(1987).Itisevidentth
4、atsedimentactsasthefinalreceptorof137Cs,showingthatfastdepollutionoftheMediterraneanstillremainsautopia.Radioactive“hotspots”wereobservedinthenorthernAegeanSeaandlowervaluesinthesouthernAegeanSeaandIonianSea.Finally,anefforttoevaluatetheriskofionizingradia
5、tion(from137Cs)tothebiotainhabitingsedimentswasmadeusingERICA.Therespectivedoseratesfortworeferenceorganisms(benthicfishandmollusks)wereestimatedtobefarbelowthescreeningdose,atwhichtheradiologicalimpactontheabundanceofthepopulationbegins.■INTRODUCTIONnear
6、-shoreintertidalsedimentsampleswerecollectedbydivers,Although137Cs(half-lifeof30.2years)wasfirstintroducedintowhereassedimentcoreswerecollectedusingaBowersand16theenvironmentbynuclearweaponstestinginthe1950sandConnelly,MarkVImulticoreranalyzer.Thesamples(
7、notearly1960s,1thelargestsourcewastheChernobylfalloutincorrectedfordecay,initially)werepreparedforactivity171986.Theaveragedensityof137CsintheAegeanSeawasmeasurementsaccordingtotheIAEAprocedures.Theresultsestimatedtobe4kBqm−2,whereasintheIonianSea,itwas2
8、.5refertobothenclosedmarineregionsandopenseakBqm−2.2Thetotalradiocesium(137Csand134Cs)inputwasenvironments(Figure1),andtheyarethereforedividedintoestimatedtobe2400TBqfortheBlackSea,3−6820TBqforfoursubregions[i.e.,northernA