铌酸锂晶体周期极化及其倍频特性研究

铌酸锂晶体周期极化及其倍频特性研究

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时间:2019-05-13

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1、南开大学硕士学位论文铌酸锂晶体周期极化及其倍频特性研究姓名:陈亚辉申请学位级别:硕士专业:光学指导教师:姚江宏20040420AbstractInthisdissertation,theperiodicallypoledcharacteristicsofZ-cutLiNb03dopedwith5tool%MgO(Mg:LN)andnear·stoichiometricLiNb03(Mg:SLN)crystalsdoped1.8t001.%MgOwereinvestigated.Thequasi·phase。matehed(QPM)secon

2、dharmonicgeneration(gHG)basedontheperiodicallypoledMg:LNandMg:SLNwerealsoinvestigated.111eresearchfindingsaredescribedinbriefasfollows:(1)ThetunabilityandtoleranceofQPMSHGinthebulkperiodicallypoledMg:LNandMg:SLNwereanalyzedThegratingperiodbandwidthandthepumpedspectralbandw

3、idth[fullwidthathalfmaximum(FWHM)]werefoundtobeinversedwiththeeffectivelengthinQPMSHG.(2)ThccharacteristicsoftheferroelectricdomaininversioninZ-catLiNb03dopedwith5m01.%MgO(Mg:LN)wereexamined.Thelowestpolarizationswitchingfield玩inMg:LNisaboutSkV/mm.Therealignmentprocessofth

4、einternalfieldinMg:LNisalsoinvestigated.Usingthespontaneousdomainsbackswitching,auniformsubmicrondomainpatterningwithaperiodof1.7umwassuccessfullyfabricated.(3)Thedomainreversalcharacteristicsofnear-stoichiometrieLiNb03wereexaminedandtheswitchfieldfor180。ferroelectricdomai

5、nreversalin*henear-stoichiomentLiNb03crystaldecreaseswith[Li]/[Li+Nb】ratio.Thcswitchfieldinthecrystal丽m[Li】/[Nb]ratioequalto49,9%wasonly3.箨kV/ram.(4)FollowingtheLivacancymodel,weexplainthereasonsofthedramaticdecreaseoftheswitchingfieldinMg:LNandMg:SLN.Wethoughtthereducibil

6、ityofLivacancyandanti—siteNbLi”defectsresultsinthedecreaseoftheswitchingfield.(5)Uniformlyperiodicdomainstructureina1.0mmthickslabofMg:LNandMg:SLNwerefabricated.UsingaQ-swilchedNd:YAGlaserasthefundamentalbeamsonreeatt.06a“nl。thegreenSHGat0.532Ⅱmwasobtainedfromperiodicallyp

7、oledMg:LNat1.亭%conversionefficiency.UsingaTi:sapphirelaser,third—orderquasi—phase·matchedsecondharmonicvioletlightgenerationWasdemonstratedinperiodicallypoledMg:SLN,withanenergyconversionefficiencyof20.5%.IIKeywords:Quasi-phase—matched(QPM)TheswitchingfieldSecondharmonicge

8、neration(SHG)PeriodicallypoledlithiumniobatedopedMgOPeriodicallypolednear-stoichiometricl

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